Study of KZn excimer molecule
Irena Labazan , Svemir Rudic, Slobodan Milosevic
Institute of Physics, P.O.Box 304, HR-10000 Zagreb, Croatia
Study of simple diatomic intermetallic excimers as building blocks of nano
structures could be important for technologies of the next century.
Most of the alkali – IIB group excimer molecules have been observed and
are well known, such as LiZn, LiCd, NaCd, KCd etc, [1]. The KZn excimer
molecule has been predicted in theoretical ab initio calculations [2],
but no experimental data were available so far. This is mainly due to the
difficulties of preparing suitable vapour mixture. Here we use heat-pipe
oven to prepare KZn amalgams with different mole ratio of potassium and
zink. With classical absorption technique and fluorescence measurements
we try to determine the best mole ratio for production of KZn.
It is very important to have small amount of potassium dimers in the
vapour mixture because of spectral overlap of KZn C-X band with K2
B-X band.
We study photoassociation (1) and photochemical (2) production of KZn
excimer:
K + Zn + hn -> KZn*
K2*+ Zn -> KZn*+ K
Very low absorption coefficient of KZn molecule is detected
with use of cavity ring down spectroscopy.
[1] S. Milosevic, Spectral Line Shapes, AIP Conf. Proc. No.328
(AIP New York, 1995), pp.391-405
[2] E. Czuchaj, F. Rebentrost, H. Stoll, H. Preuss, Chem. Phys.
Letters 218 (1994) 454-461